Gold nanoparticle liquid crystal composites as a tunable nonlinear medium

We investigate the nonlinearity of a liquid crystal cell doped with gold nanoparticles by considering their selective absorption. Such nonlinearities are promising for optical processing applications and optical limiters. Systems displaying thermal nonlinearities are particularly attractive as the maximum nonlinearity may occur in the absence of an applied field and additionally this nonlinearity can be controlled by the reorientation of the liquid crystal. We show that there exists a theoretical optimum concentration of absorbers, which maximizes the nonlinearity. Further we show that the nonlinearity of the system can be tuned by the reorientation of the liquid crystal host, with the nonlinearity decreasing from 9 × 10-5 cm2/W to zero by the application of a magnetic field of the order of 0.01 Tesla. This allows a fine control of the diffraction efficiency and, in principle, many other nonlinear effects

Large effect of a small bias field in liquid-crystal magnetic transitions

Most liquid crystals show low sensitivity to magnetic field. However, in this paper we show that a small bias magnetic field not only breaks the symmetry of the ground state, but also plays a crucial role in facilitating the reorientation induced by a large test magnetic field. In particular, a small bias field may alter significantly the strength of the test field needed to observe a given reorientation of the liquid crystal. Moreover, the bias field interacts with other symmetry breaking features of the cell, e.g., pretilt, to change also the qualitative features of the equilibrium state

Voltage transfer function as an optical method to characterize electrical properties of liquid crystal devices

The voltage transfer function is a rapid and visually effective method to determine the electrical response of liquid crystal (LC) systems using optical measurements. This method relies on cross-polarized intensity measurements as a function of the frequency and amplitude of the voltage applied to the device. Coupled with a mathematical model of the device it can be used to determine the device time constants and electrical properties. We validate the method using photorefractive LC cells and determine the main time constants and the voltage dropped across the layers using a simple nonlinear filter model

Self-induced liquid crystal q-plate by photoelectric interface activation

International audienceHere, we report on the experimental demonstration that highly efficient self-induced spin-orbit optical vortex generation can be achieved by using standard liquid crystal materials and surface treatment agents. This is done by revisiting the recent attempt by Zolot’ko and coworkers to produce self-induced liquid crystal vortex plates using the dc electric field [I. A. Budagovsky, S. A. Shvetsov, and A. S. Zolot’ko, Mol. Cryst. Liq. Cryst. 637, 47 (2016)] that remains, so far, limited to moderate efficiencies. The phenomenon is the result of the self-back-action of light arising from the spontaneous creation of a liquid crystal topological defect. These results demonstrate photo-electric interface activation as a candidate towards the development of a self-adapted spinorbit photonic toolbox, thus enabling agile management of the orbital angular momentum of light

Light-activated modulation and coupling in integrated polymer-liquid crystal systems

We explore the transfer of an incident light pattern onto the liquid crystal (LC) bulk in a photorefractive cell through an integrated photoconducting layer that modulates the electric field applied to the device. The electrical properties and the strength of modulation are investigated as a function of the incident light intensity as well as the frequency and amplitude of the applied voltage, for two LCs with very different electrical conductivity. A simplified electrical model of the cell is proposed, demonstrating that the LC conductivity is a key factor determining the beam-coupling strength

100 GHz electrically tunable planar Bragg grating via nematic liquid crystal overlay towards reconfigurable WDM networks

Novel liquid crystal-based integrated optical devices with >140GHz electrical tuning are presented for application towards reconfigurable wavelength division multiplexing (WDM) networks. Initial results with Bragg wavelength tuning covering five 25GHz WDM channel spacing have been achieved with 170V (peak-to-peak) sinusoidal voltages applied across electro-patterned ITO-covered glass electrodes placed 60µm apart. These prototype devices were fabricated using direct UV grating writing, with an evanescent field coupling into a liquid crystal overlay through an etched window. Electrically controlled liquid crystal birefringence modifies the waveguide effective index, resulting in Bragg wavelength shift. Merck 18523 nematic liquid crystals are used, exhibiting compatible refractive index values to that of silica (no=1.44, ne=1.49 at lambda=1550nm). Homeotropic alignment of the liquid crystal is provided by application of a surfactant layer.The inherent refractive index sensitivity of our etched direct-UV-written structures allows observation of previously unreported liquid crystal surface-behaviour, such as multi-threshold points during variation of the applied field. Continued optimisation based on evanescent field penetration, electrode layout, and surface interaction will allow implementation towards a variety of novel liquid crystal applications and devices. For example, a cascaded architecture of these integrated liquid crystal devices operating at different Bragg wavelengths would pave the way towards true colorless add/drop modules for dense optical networks

Topological learning for the classification of disorder: an application to the design of metasurfaces

Structural disorder can improve the optical properties of metasurfaces, whether it is emerging from some large-scale fabrication methods, or explicitly designed and built lithographically. Correlated disorder, induced by a minimum inter-nanostructure distance or by hyperuniformity properties, is particularly beneficial in some applications such as light extraction. We introduce numerical descriptors inspired from topology to provide quantitative measures of disorder whose universal properties make them suitable for both uncorrelated and correlated disorder, where statistical descriptors are less accurate. We prove theoretically and experimentally the accuracy of these topological descriptors of disorder by using them to design plasmonic metasurfaces of controlled disorder, that we correlate to the strength of their surface lattice resonances. These tools can be used for the fast and accurate design of disordered metasurfaces, or to help tuning large-scale fabrication methods.Comment: 6 figure